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81.
Background River and lake sediments constitute complex and difficult analytical samples. On the other hand, sediments play a fundamental
role in the distribution of toxic compounds in aquatic systems and in the evaluation of the current state and the course of
changes taking place in the environment.
Among elements present in the environment in trace concentrations, but having well-elaborated toxic properties, one of most
dangerous is arsenic. The element occurs in the environment in several chemical forms, predominant are inorganic forms of
As(V) and As(III), and methylated forms such as monomethylarsonic acid (MMAA) and dimethylarsinic acid (DMAA).
Objectives Reported herein are experiments, which were undertaken with the aim of examining the dynamics of arsenic sorption in sediments
and its dependence on speciation of the element and the pH in the environment. Simultaneously, influence of organic matter
content and chemical composition of the sediments on As sorption, were investigated.
Methods Sediment samples (upper 10 cm layer) were collected from three sites located in the vicinity of Cracow:
Using XRD and IR methods, mineral composition of sediments was analysed. Concentrations of iron, manganese, aluminium and
arsenic as well as organic matter content in solid samples were analysed.
Sorption experiment 100 g of dry sediment sample was placed in a 400 ml volume glass beaker. 300 ml of arsenic containing solution was poured
into the beaker. Every 30 min (total experiment time span equalled 7 to 7.5 hours), 0.5 ml of the suspension’ (the beaker
content was constantly mixed) was collected and centrifuged, and the concentration of arsenic was determined in the supernatant.
In the series of experiments, solution contained about 0.05 μg/ml of arsenic in organic (DMAA) and inorganic forms, at different
pH values — 3, 5, 7 and 9.
Results and Discussion Examined sediments of Vistula river and Dobczyce Lake were characterised by relatively high concentrations of arsenic, iron,
manganese and aluminium.Rudawa river. At pH 3, the concentration of inorganic As in solution decreased from an initial value of 0.049 μg/ml to 0.012 μg/ml in
7.5 hours time. The same decreasing tendency was found at pH 5 (initial value 0.046 μg/ml, after 7.5 hours - 0.015 μg/ml).
Less distinct sorption effects were noted at pH 7 and 9.
Vistula river. At all pH values, a very significant decrease of inorganic As concentration up to 80% of the initial value, as well as a
short time of achieving an equilibrium state (1 – 2.5 hours), was found.
Dobczyce lake. Inorganic As was distinctly accumulated in sediments at pH 3 (decrease of As concentration in solution from 0.052 to 0.007
μg/ml after 7.5 hours of the experiment) and at pH 5. At pH 7, about 40% of As was accumulated in sediments (solution As concentration
decrease from 0.050 to 0.030). Only 20% of As adsorbed on sediments at pH 9.Very weak accumulation of organic form of As (DMAA)
was found in all examined sediments at pH 3 and 5. At higher pH values no sorption was registered.
Conclusions The following facts were established:
Recommendations The presented method of analysis of As sorption in sediments and results visualization (based on a newly defined coefficient)
provides a useful tool for the characterization of sorptive properties of sediments and may be used for other compounds as
well. Crucial, functional information — how much of a given element may be accumulated in sediments at a certain pH — is obtained
without digestion of the sediment sample, in an experiment taking less than one day. 相似文献
| • | Rudawa river — 37 km long river, flowing mainly through the suburban area; |
| • | Vistula river — heavily contaminated, main Polish river; |
| • | Dobczyce reservoir — artificial reservoir on Raba river, total capacity of 125,000,000 m3, supplying about 60% of drinking water to the city of Cracow. |
| • | inorganic form of arsenic was effectively accumulated in all analysed sediments; |
| • | inorganic As sorption in sediments strongly depended on pH — for sediments of Rudawa river and Dobczyce lake, the highest sorption was found at pH 3, and a decrease of accumulated As was noted with an increase of pH (at pH 9, the lowest amount of As was immobilised in sediments); in the case of Vistula river sediments, a reverse tendency was found; |
| • | organic form of arsenic (DMAA) was accumulated only at pH 3 in all sediments and less significantly at pH 5 (Vistula river sediments); no sorption of that form of As was found in the other sediment samples; |
| • | state of equilibrium (no change in inorganic As concentration in liquid medium) was achieved in 1 hour for Vistula river sediments, after about 2 hours for Rudawa river and after about 4 hours for Dobczyce lake sediments. |
82.
清涧河流域水土流失严重。年侵蚀模数在１００００ｔ／ｋｍ２以上。自５０年代初开展水土保持工作，截至１９８９年底止，共治理水土流失面积２２０４．０７ｋｍ２，治理程度达５０．６７％，流域输水输沙明显减少。分析表明：清涧河水沙减少受降雨和流域治理的共同影响，与１９６９年以前相比，７０年代年均减沙１５．４％，８０年代年均减沙７１．３％。在减沙量中，降雨偏枯影响７０年代占１４．６％～２８．２％，８０年代占３６．９％～４１．８％；流域治理减沙量７０年代占７１．８％～８５．５％，８０年代占５８．２％～６３．１％。同时，流域治理减水量也由７０年代的１８．２％～３３．９％增加到８０年代的４２．９％～４７．７％。 相似文献
83.
84.
85.
Presently, the soil water balance of flood‐influenced soils in fluvial plains is insufficiently described. The new development of a weighable groundwater lysimeter is the basis for recording the water‐balance components precipitation, evapotranspiration, groundwater recharge, capillary rise, and interaction with the water course. Soil‐hydrologic measuring setups at two floodplain sites of the Elbe river serve for direct comparability of lysimeter measurements with data obtained on site. A groundwater control was designed for lysimeters that automatically adjusts the current groundwater level at the floodplain measuring setups and quantifies inflow into or outflow from the lysimeter. It turned out that the lysimeter developed is capable of identifying the individual water‐balance quantities at high accuracy. Contrary to previous assumptions, it was possible to prove groundwater recharge for the floodplain sites. 相似文献
86.
景观生态学在河流生态修复中的应用 总被引：15，自引：0，他引：15
景观生态学强调景观的时空变化,非常适于评价和定量描述河流的变化,已被广泛用来管理和修复河流生态系统,对我国大规模的水土保持生态环境建设将产生深远而重要的影响。基于景观生态学的预案方法是生态修复的有效工具。 相似文献
87.
塔里木河下游应急生态输水工程改善了该区水资源匮乏的现状,地下水的平均水位从输水前的8.25m升至输水后的4.13m。相应地,地表植被也出现明显的响应。但是,在不同河段由于过水时间、耗水量等因素的差异,造成输水后水位差异较大。以既能减少地下水强烈蒸发返盐,又不造成土壤干旱而影响植物生长的合理生态水位作为评价标准,对输水后不同河段的地下水位进行分析。结果显示,目前英苏—阿拉干段的地下水位2.97～4.8m是比较理想的水位;大西海子—英苏段水位较高,可能出现次生盐渍化;阿拉干—台特玛湖段地下水位太低,不利于植被的自然恢复。 相似文献
88.
三种网格的农田防护林防止土壤风蚀的效应研究 总被引：8，自引：0，他引：8
在山东省夏津县黄河故道冲积沙地建立土壤风蚀试验区,采用标尺法对3种网格的农田防护林和对照地的土壤风蚀量进行观测,测定结果表明:农田防护林网可明显减少风蚀损失,其中,130m×300m林网相对于对照减少土壤风蚀量81%,260m×300m林网相对于对照减少78%,300m×400m林网相对于对照减少75%,即随着网格面积的增加对风蚀量的影响越来越小。同时,土壤风蚀程度与测定期间日平均风速>4 m/s的出现频率有密切关系,土壤风蚀量与风速之间的最佳拟合关系为幂函数关系,二者之间呈正相关关系,相关系数在0.95以上。黄河故道冲积沙地农田防护林网对5.0~5.9 m/s范围内的风速引起的土壤风蚀防治效果最好。 相似文献
89.
不同经营类型红松林对汤旺河流域土壤性质的影响 总被引：8，自引：2，他引：8
通过实地调查与试验分析，研究了汤旺河流域4种经营类型红松林对土壤性质的影响情况。结果表明：在研究地区无论土壤pH、土壤有机质，还是土壤养分和土壤物理性质，白桦与红松天然更新形成的混变林和白桦与红松人工造林形成的混交林都较红松人工纯林优越，维护林分土壤地力及涵养水分的功能强。而红松人工纯林较原始红松林和两种白桦红松混交林维护地力及涵养水分功能弱。研究结果为汤旺河流域森林恢复与重建提供了科学合理的途径。 相似文献
90.
侯庆春先生，研究员。1943年出生于吉林省吉林市，1965年毕业于东北林学院林学系，同年分配到中国科学院水利部水土保持研究所工作至今。30多年来一直在黄土高原从事森林生态学和造林学方面的研究工作，研究领域涉及到黄土高原造林的诸多领域，先后对黄土高原林草地土壤水分特征及区域分布、飞机播种造林种草技术，抗旱防风集流造林技术，区域林业、小流域综合治理，低产林改造等方面进行了深入系统的研究。 相似文献